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Oxygen electroreduction catalysed by laccase wired to gold nanoparticles via trinuclear copper cluster

dc.contributor.authorDagys, Marius
dc.contributor.authorLaurynėnas, Audrius
dc.contributor.authorRatautas, Dalius
dc.contributor.authorKulys, Juozas
dc.contributor.authorVidžiūnaitė, Regina
dc.contributor.authorTalaikis, Martynas
dc.contributor.authorNiaura, Gediminas
dc.contributor.authorMarcinkevičienė, Liucija
dc.contributor.authorMeškys, Rolandas
dc.contributor.authorShleev, Sergey
dc.date.accessioned2023-09-18T16:46:39Z
dc.date.available2023-09-18T16:46:39Z
dc.date.issued2017
dc.identifier.issn1754-5692
dc.identifier.urihttps://etalpykla.vilniustech.lt/handle/123456789/116496
dc.description.abstractSpecific wiring of biocatalysts par excellence, viz. redox enzymes, to the electrode can be exploited in fabrication of high-performance bioelectronic devices. Here we report oxygen electroreduction catalysed by Didymocrea sp. J6 laccase wired to the gold nanoparticles via trinuclear copper cluster. Bypassing the intramolecular electron transfer, which under certain conditions is the rate limiting step of oxygen bioelectroreduction, has resulted in fabrication of a high current density biocathode based on high redox potential laccase, which is able to operate in electrolytes at a broad pH range in the presence of high fluoride concentrations.eng
dc.formatPDF
dc.format.extentp. 498-502
dc.format.mediumtekstas / txt
dc.language.isoeng
dc.relation.isreferencedbyCurrent Contents
dc.relation.isreferencedbyPubMed
dc.relation.isreferencedbyScopus
dc.relation.isreferencedbyCompendex
dc.relation.isreferencedbyINSPEC
dc.relation.isreferencedbyScience Citation Index Expanded (Web of Science)
dc.source.urihttp://pubs.rsc.org/en/content/articlehtml/2017/ee/c6ee02232d
dc.subjectFM02 - Energijos šaltinių medžiagos ir technologijos / Materials and technologies of energy sources
dc.titleOxygen electroreduction catalysed by laccase wired to gold nanoparticles via trinuclear copper cluster
dc.typeStraipsnis Web of Science DB / Article in Web of Science DB
dcterms.references44
dc.type.pubtypeS1 - Straipsnis Web of Science DB / Web of Science DB article
dc.contributor.institutionVilniaus universitetas
dc.contributor.institutionVilniaus universitetas Vilniaus Gedimino technikos universitetas
dc.contributor.institutionMalmö University Kurchatov NBICS Centre
dc.contributor.facultyFundamentinių mokslų fakultetas / Faculty of Fundamental Sciences
dc.subject.researchfieldN 004 - Biochemija / Biochemistry
dc.subject.researchfieldT 005 - Chemijos inžinerija / Chemical engineering
dc.subject.ltspecializationsL102 - Energetika ir tvari aplinka / Energy and a sustainable environment
dc.subject.enLaccase
dc.subject.enGold nanoparticle
dc.subject.enBiofuel cells
dc.subject.enTrinuclear copper cluster
dcterms.sourcetitleEnergy & environmental science
dc.description.issueIss. 2
dc.description.volumeVol. 10
dc.publisher.nameRoyal Society of Chemistry
dc.publisher.cityCambridge
dc.identifier.doi000395679100006
dc.identifier.doi10.1039/C6EE02232D
dc.identifier.elaba18917312


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